Angle-resolved photoemission study of USb2 the 5f band struc(7)

2021-04-05 23:36

Single crystal antiferromagnetic USb2 was studied at 15K by angle-resolved photoemission with an overall energy resolution of 24 meV. The measurements unambiguously show the dispersion of extremely narrow bands situated near the Fermi level. The peak at th

below the Fermi level the electronic band structure of USb2 is dominated by U6d and U5f states.

The normal emission PES spectra measured for hν = 34 eV (Fig.2a) shows one sharp feature situated near the Fermi edge. The rest of the spectrum remains completely flat, which is an evidence of a very clean, high quality sample surface resulting in very well defined incidence and emission angles. The peak near the Fermi edge, which was interpreted so far as the U5f-conduction band hybridized narrow band, changes its position from 37 meV for θ = 00 to 23 meV for θ = 60 and 70 giving evidence of a 14 meV dispersion (Fig. 2b). For θ = 50 the FWHM of this peak starts growing from 24 meV for lower angles, up to 48 meV for θ = 70. The given FWHM values include the instrumental resolution and thus the natural line width is extremely sharp (as demonstrated in the detailed analysis of Fig.1). When fitting the data we use a Gaussian function for experimental resolution and a Lorentzian function for the natural line width. For θ = 80 and 90 we see two structures in the Fermi level region. It appears that the increase in width away from normal is a result of two states with different dispersions.

A large dispersion (about 270 meV) is shown in the structure marked as

B in Fig. 2b, which appears at 470 meV below the Fermi level for θ = 40. The intensity of this structure grows gradually up to θ = 90, whereas the binding energy shifts downwards and for θ = 90 it is situated at 200 meV.

The PES spectra taken for hν = 43 eV (Fig.3) also shows dispersion of peak A, which changes the energy position from 34 meV (θ = 00) to 48 meV (θ = 60). We can not see two peaks for θ = 60, but the FWHM is almost twice of that for θ = 50, which suggests an additional contribution for higher angles. The structure B appears for θ = 20 at a binding energy of 410 meV and changes its binding energy position to 234 meV for θ = 60.

Photoemission data for hν = 60 eV (Fig.4) show both A and B structures even in the normal emission spectrum. The dispersion of peak A in this case is 14 meV, the A position for θ = 00 is 67 meV and for θ = 100 is 81 meV below E F. The structure B is

7


Angle-resolved photoemission study of USb2 the 5f band struc(7).doc 将本文的Word文档下载到电脑 下载失败或者文档不完整,请联系客服人员解决!

下一篇:一年级数学下册100以内加减法口算练习题连加连减

相关阅读
本类排行
× 注册会员免费下载(下载后可以自由复制和排版)

马上注册会员

注:下载文档有可能“只有目录或者内容不全”等情况,请下载之前注意辨别,如果您已付费且无法下载或内容有问题,请联系我们协助你处理。
微信: QQ: